Ferrocenes: Homogeneous Catalysis/Organic by Antonio Togni, Tamio Hayashi

By Antonio Togni, Tamio Hayashi

This publication captures the multidisciplinary nature of ferrocene learn. Well-referenced and written by means of major specialists within the box, it's a welcome resource of in-depth info for graduate scholars and pros in natural, organometallic, and polymer chemistry, in addition to in fabrics technology.

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These atomic and molecular motions appear to be related to the coordination modes of the ligand and to the metal geometry. In contrast to the unidentate and open-bridging dppf complexes, the chelates generally exhibit a greater extent of ring tilting but minimal divergence of the phosphorus atoms. 13 8, (Table 1-2). Other restrained systems like the doubly, quasi-closed and closed bridging complexes also exhibit similar tilts to those of the chelates. There is also evidence that Cp ring tilting is most marked among the square-planar chelates.

M. Draper, C. E. Housecroft, A. L. Rheingold, J. Organomet. Chem. 1992, 435, 9-20. diamine (TMEDA) [18, 191. In spite of its early discovery, the development of dppf chemistry took off in a significant way only in the 1980s. Since then, a multitude of dppf complexes has been synthesized (Table 1-1) and the conformational flexibilityand catalytic activity of dppf itself have been widely explored. Coordination complexes of dppf are generally prepared by the direct reaction of dppf with binary compounds [20, 211 or other primary forms of Lewis acids [22]..

52] G. Pilloni, R. Graziani, B. Longato, B. Corain, Znorg. Chim. Acta 1991, 190, 165- 167. [53] C. Vogler, W. Kaim, J . Organomet. Chem. 1990, 398, 293-298. -P. -Y. Zhou, T. C. W. Mak, T. S. A. Hor, J . Chem. , Dalton Trans. 1994, in press. -P. Neo, T. S. A. -Y. Zhou, T. C. W. Mak, J. Organomet. Chem. 1994,464,113 - 119. [56] T. S. A. Hor, S. P. Neo, C. S. Tan, T. C. W. Mak, K. W. P. -J. Wang, Znorg. Chem. 1992, 31, 4510-4516. [57] A. Houlton, R. M. G. Roberts, J. Silver, R. V. Parish, J . Organornet.

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